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Global analysis of continental boundary layer new particle formation based on long-term measurements

Atmospheric new particle formation (NPF) is an important phenomenon in terms of global particle number concentrations. Here we investigated the frequency of NPF, formation rates of 10 nm particles, and growth rates in the size range of 10-25 nm using …

Predicting atmospheric particle formation days by Bayesian classification of the time series features

Atmospheric new-particle formation (NPF) is an important source of climatically relevant atmospheric aerosol particles. NPF can be directly observed by monitoring the time-evolution of ambient aerosol particle size distributions. From the measured …

Exploring non-linear associations between atmospheric new-particle formation and ambient variables: a mutual information approach

Atmospheric new-particle formation (NPF) is a very non-linear process that includes atmospheric chemistry of precursors and clustering physics as well as subsequent growth before NPF can be observed. Thanks to ongoing efforts, now there exists a …

The role of H2SO4-NH3 anion clusters in ion-induced aerosol nucleation mechanisms in the boreal forest

New particle formation (NPF) provides a large source of atmospheric aerosols, which affect the climate and human health. In recent chamber studies, ion-induced nucleation (IIN) has been discovered as an important pathway of forming particles; …

Comprehensive analysis of particle growth rates from nucleation mode to cloud condensation nuclei in boreal forest

Growth of aerosol particles to sizes at which they can act as cloud condensation nuclei (CCN) is a crucial factor in estimating the current and future impacts of aerosol-cloud-climate interactions. Growth rates (GRs) are typically determined for …

Atmospheric new particle formation from sulfuric acid and amines in a Chinese megacity

Atmospheric new particle formation (NPF) is an important global phenomenon that is nevertheless sensitive to ambient conditions. According to both observation and theoretical arguments, NPF usually requires a relatively high sulfuric acid (H2SO4) …

Observations of biogenic ion-induced cluster formation in the atmosphere

A substantial fraction of aerosols, which affect air quality and climate, is formed from gaseous precursors. Highly oxygenated organic molecules (HOMs) are essential to grow the newly formed particles and have been evidenced to initiate ion-induced …

Atmospheric new particle formation at the research station Melpitz, Germany: connection with gaseous precursors and meteorological parameters

This paper revisits the atmospheric new particle formation (NPF) process in the polluted Central European troposphere, focusing on the connection with gas-phase precursors and meteorological parameters. Observations were made at the research station …

Influence of temperature on the molecular composition of ions and charged clusters during pure biogenic nucleation

It was recently shown by the CERN CLOUD experiment that biogenic highly oxygenated molecules (HOMs) form particles under atmospheric conditions in the absence of sulfuric acid, where ions enhance the nucleation rate by 1-2 orders of magnitude. The …

Observations of ozone depletion events in a Finnish boreal forest

We investigated the concentrations and vertical profiles of ozone over a 20-year period (1996-2016) at the SMEAR II station in southern Finland. Our results showed that the typical daily median ozone concentrations were in the range of 20-50 ppb with …